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已經(jīng)被收錄 High and selective CO2 uptake in a nitrogen-rich pillar-layered metal organic framework 作者:Chen, C (Chen, Chao)[ 1 ] ; Jia, MF (Jia, Minfeng)[ 1 ] ; Wang, G (Wang, Gang)[ 1 ] ; Li, XL (Li, Xiaoli)[ 1 ] ; Li, SM (Li, Shimin)[ 1 ] RSC ADVANCES 卷: 5 期: 127 頁: 104932-104935 DOI: 10.1039/c5ra22144g 出版年: 2015 查看期刊信息 摘要 A nitrogen-rich pillar-layered metal organic framework, Co(Imda)(4,4'-bpy), comprising cobalt(II) clusters interconnected by imidazole-4,5-dicarboxylic acid and 4,4'-bipyridyl groups was synthesized, and characterized by powder X-ray diffraction, N-2 adsorption-desorption measurements, thermogravimetric analysis, and scanning electron microscopy. This material was firstly investigated for CO2 capture. It exhibited several outstanding attributes as a CO2 adsorbent: high CO2 uptake (135 mg g(-1) at 298 K, 1 bar), good separation selectivity against N-2 (CO2/N-2 selectivity of ca. 18 at 298 K, 1 bar), fast adsorption kinetics (saturation within 10 min), easy regeneration (298 K, argon purge) and excellent stability in moisture and during consecutive adsorption-desorption cycles. 關(guān)鍵詞 KeyWords Plus:CARBON-DIOXIDE; ROOM-TEMPERATURE; GAS SEPARATION; CAPTURE; ADSORPTION; NETWORKS; CAPACITY; SORPTION; CO2/CH4; STORAGE 作者信息 通訊作者地址: Chen, C (通訊作者) Xinyang Normal Univ, Coll Chem & Chem Engn, Xinyang 464000, Henan Province, Peoples R China. 地址: [ 1 ] Xinyang Normal Univ, Coll Chem & Chem Engn, Xinyang 464000, Henan Province, Peoples R China 電子郵件地址:chenchao@xynu.edu.cn 基金資助致謝 基金資助機(jī)構(gòu) 授權(quán)號(hào) Key Project of Scientific and Technological Research of Henan Provincial Committee of Education 13A150757 查看基金資助信息 出版商 ROYAL SOC CHEMISTRY, THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND 類別 / 分類 研究方向:Chemistry Web of Science 類別:Chemistry, Multidisciplinary 文獻(xiàn)信息 文獻(xiàn)類型:Article 語種:English 入藏號(hào): WOS:000366865900038 ISSN: 2046-2069 期刊信息 Impact Factor (影響因子): Journal Citation Reports® 其他信息 IDS 號(hào): CZ1KY Web of Science 核心合集中的 "引用的參考文獻(xiàn)": 21 Web of Science 核心合集中的 "被引頻次": 0 |
2樓2016-03-11 11:25:58
ccloveshumin
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