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Rational design of a novel indole-based microporous organic polymer: enhanced carbon dioxide uptake via local dipole-pi interactions 作者:Chang, GJ (Chang, Guanjun)[ 1 ] ; Shang, ZF (Shang, Zhenfang); Yu, T (Yu, Tao); Yang, L (Yang, Li)[ 1 ] JOURNAL OF MATERIALS CHEMISTRY A 卷: 4 期: 7 頁: 2517-2523 DOI: 10.1039/c5ta08705h 出版年: 2016 查看期刊信息 摘要 An indole-based microporous organic polymer (PINK) has been obtained by the condensation polymerization of 1,3,5-tris-(4-fluorobenzoyl) benzene with 3,3'-diindolylmethane via a catalyst-free nucleophilic substitution reaction. Due to the local dipole-p interactions between indole and carbon dioxide (CO2), the uptake capacity for CO2 reaches up to 16.0 wt% (1.0 bar, 273 K), and the high (CO2/N-2 = 15, CO2/CH4 = 32) selectivities of the polymer make it a promising material for potential application in gas separation. Furthermore, the hydrogen storage is up to 2.48 wt% (1.0 bar, 77 K). In comparison to the reported porous organic polymers, the preparative strategy exhibits cost-effective advantages, which are essential for scale-up preparation. Its good performance for H-2 storage and CO2 separation suggests that PINK with a large specific surface area shows potential use in clean energy applications and the environmental field. 關(guān)鍵詞 KeyWords Plus:HYDROGEN STORAGE; SURFACE-AREA; INTRINSIC MICROPOROSITY; ENERGY APPLICATIONS; CO2 CAPTURE; CATION-PI; ADSORPTION; FRAMEWORKS; NETWORKS; POROSITY 作者信息 通訊作者地址: Chang, GJ; Yang, L (通訊作者) 顯示增強(qiáng)組織信息的名稱 Southwest Univ Sci & Technol, State Key Lab Cultivat Base Nonmetal Composite &, Mianyang 621010, Peoples R China. 地址: 顯示增強(qiáng)組織信息的名稱 [ 1 ] Southwest Univ Sci & Technol, State Key Lab Cultivat Base Nonmetal Composite &, Mianyang 621010, Peoples R China 顯示增強(qiáng)組織信息的名稱 [ 2 ] Southwest Univ Sci & Technol, Sch Mat Sci & Engn, Mianyang 621010, Peoples R China 電子郵件地址:gjchang@mail.ustc.edu.cn; yanglichem628@126.com 基金資助致謝 基金資助機(jī)構(gòu) 授權(quán)號(hào) National Natural Science Foundation of China 21202134 11447215 21504073 Project of Research and Development of Applied Technology of Mianyang City of China 14G-01-3 Open Project of State Key Laboratory Cultivation Base for Nonmetal Composites and Functional Materials 11zxfk26 14tdfk03 查看基金資助信息 出版商 ROYAL SOC CHEMISTRY, THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND 類別 / 分類 研究方向:Chemistry; Energy & Fuels; Materials Science Web of Science 類別:Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary 文獻(xiàn)信息 文獻(xiàn)類型:Article 語種:English 入藏號(hào): WOS:000369665800017 ISSN: 2050-7488 eISSN: 2050-7496 QQ截圖20170624090615.png |
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