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Chemical Reviews最新綜述：異相納米復(fù)合物催化劑中的催化協(xié)同作用 已有32人參與
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最新一期的頂級(jí)綜述雜志Chemical Reviews刊發(fā)了由中科院上海硅酸鹽研究所施劍林研究員撰寫的綜述，題目為On the Synergetic Catalytic Effect in Heterogeneous Nanocomposite Catalysts，介紹了異相納米復(fù)合物催化劑的各種合成方法，并著重綜述了納米復(fù)合物中各組份活性物質(zhì)在催化反應(yīng)中的協(xié)同效應(yīng)。全文43頁(yè)，引文376篇。 1. Introduction 1.1. Definition of the “Synergetic Catalytic Effect” in Heterogeneous Composite Catalysts 1.2. Scope of the Present Review 2. Synthesis of Nanocomposite Catalysts Focused on Mesostructured Composites with a Crystallized Framework 2.1. General Description of Chemical Routes for Synthesizing Nanocomposite Catalysts 2.2. Soft Templating Routes for the Mesoporous Oxides, Mesostructured Zeolites, and Nanocomposites 2.3. Replication Routes for Crystallized Mesoporous Oxides and Binary Mesoporous Composites 2.4. Template-free Routes for Mesoporous Metal Oxides and Composites 2.5. Postencapsulation Routes for the Guest-Loaded Mesoporous Composites 3. Synergetic Catalytic Effects 3.1. One Component Activation by the Other between Two Catalytic Components 3.1.1. Synergetic Effect Proposals 3.1.2. CO Oxidation by Mesoporous CuO/CeO2 Composite Catalysts via Strong Metal–Semiconductor Interaction (SMSI) 3.1.3. Methanol Synthesis by Cu/ZnO-Based Catalysis via Strong Metal–Semiconductor Interaction (SMSI) 3.1.4. Suzuki/Heck C–C Coupling by Mesostructured Pd/NiFe2O4 Composite Catalysts 3.1.5. Selective Oxidation of Organics by Au/TiO2 and Au/CeO2 Nanocomposite Catalysts 3.1.6. Organics Degradation by Au/TiO2, TiO2/Carbon, and TiO2/Semiconductor Nanocomposite Photocatalysts 3.2. Successive Catalytic Functioning of Two Components in Multistep Reactions 3.2.1. Synergetic Effect Proposals 3.2.2. Henry and Adol Condensation Reactions by Mesoporous Acid–Base Catalysts 3.2.3. Dye Degradation by Fe-Doped Mesoporous Zeolite 3.2.4. Ammonia Selective Catalytic Oxidation (SCO) to Nitrogen by a Mesostructured CuO/RuO2 Composite 3.3. Degradation Prevention of the Main Catalyst(s) by Secondary Component(s) for Sustained Catalytic Reactions 3.3.1. Synergetic Effect Proposals 3.3.2. H2 Electro-oxidation by Mesostructured Pt/WO3 Composite Catalysts 3.3.3. Methanol Electro-oxidation by Mesostructured Pt/WO3 Composite Catalysts 3.4. Reactant Storage/Release by the Catalytic Assistants in Multireactant Redox Reactions Catalyzed by Tricomponent Catalysts 3.4.1. Synergetic Effect Proposal 3.4.2. Oxygen Storage/Release in Three Way Catalysis for Automobile Exhaust Purification 3.4.3. Promoted Redox Reaction between CO and NO and between NO and C3H6 by a Tricomponent Catalyst with an Oxygen Storage Support 4. Further Discussions: Role of Interface and Mesostructure in Synergetic Catalytic Effects 4.1. Role of Interface Formation and Contact Angle between Components in the Synergetic Catalytic Effects 4.2. Advantages of Mesostructured Composites for the Synergetic Effects 5. Conclusions and Outlook cr-2012-002752_0046.gif [ 來(lái)自科研家族 材料家族 ] |
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