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| 【獎(jiǎng)勵(lì)】 本帖被評(píng)價(jià)160次，作者shileijerry增加金幣 126.6 個(gè) | ||||||||||||||||||
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分子納米動(dòng)力學(xué)Molecular Nano Dynamics
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Molecular Nano Dynamics [2 Vols] Molecular Nano Dynamics......Page 5 Preface......Page 19 About the Editors......Page 21 List of Contributors for Both Volumes......Page 25 Volume I: Spectroscopic Methods and Nanostructures......Page 1 Contents to Volume 1......Page 7 Part One: Spectroscopic Methods for Nano Interfaces......Page 35 1.1 Introduction......Page 37 1.2.1 Raman Spectroscopy......Page 38 1.3 Theoretical Approaches......Page 40 1.4.1 STM Combined with Raman Spectroscopy......Page 42 1.4.2 STM Combined With Fluorescence Spectroscopy......Page 46 1.5 Future Prospects......Page 47 References......Page 50 2.1 Introduction......Page 53 2.2 Surface Plasmon Polaritons......Page 54 2.3 Near-Field Optical Microscopy Using a Metallic Nano-Tip......Page 56 2.4 Tip-Enhanced Near-Field Raman Spectroscopy and Imaging......Page 58 2.4.2 Near-Field Nano-Raman Microscopy......Page 59 2.4.3 Tip-Enhanced Near-Field Raman Spectroscopy and Imaging......Page 60 2.5 Tip Effect on Near-Field Raman Scattering......Page 64 References......Page 70 3.1 Introduction......Page 73 3.2 Near-Field Spectroscopic Method......Page 74 3.4 Wavefunction Images of Plasmon Modes of Gold Nanorod — Near-Field Transmission Method......Page 76 3.5 Ultrafast Time-Resolved Near-Field Imaging of Gold Nanorods......Page 79 3.6 Near-Field Two-Photon Excitation Images of Gold Nanorods......Page 81 3.7 Enhanced Optical Fields in Spherical Nanoparticle Assemblies and Surface Enhanced Raman Scattering......Page 82 3.8 Concluding Remarks......Page 85 References......Page 86 4.1 Introduction......Page 89 4.2.2 Near-Field Optical Microscopy......Page 90 4.2.3 Structure of a Single Polymer Chain......Page 92 4.3.2 Fluorescence Depolarization Method......Page 95 4.3.3 Dynamics of a Polymer Brush......Page 97 4.4 Summary......Page 101 References......Page 102 5.1 Introduction......Page 105 5.2.1 Brief Description of SFG......Page 106 5.2.2 Origin of SFG Process......Page 107 5.2.3 SFG Spectroscopy......Page 108 5.2.4.1 Laser and Detection Systems......Page 111 5.2.4.2 Spectroscopic Cells......Page 112 5.3.2 Results and Discussion......Page 114 5.3.3 Conclusions......Page 117 5.4.1 Introduction......Page 118 5.4.2 Results and Discussion......Page 119 5.4.3 Conclusions......Page 122 5.5.1 Introduction......Page 123 5.5.2 Results and Discussions......Page 124 5.5.3 Conclusions......Page 126 5.6.2 Enhancement of Hyper-Raman Scattering Intensity......Page 128 5.7 General Conclusion......Page 130 References......Page 131 6.1 Why Buried Interfaces?......Page 137 6.2 Optical Transitions......Page 138 6.3 Experimental Scheme......Page 140 6.4 Application to a Liquid Surface......Page 141 6.5 Application to a Liquid/Liquid Interface......Page 142 6.6 Applications to Solid Surfaces......Page 143 6.7 Frequency Domain Detection......Page 146 References......Page 147 7.1.1 Weak Force Measurements......Page 151 7.1.2 Potential Analysis Method Using Photon Force Measurement......Page 152 7.2.1 Two-Beam Photon Force Measurement System......Page 155 7.2.2 Potential Analysis Method for Hydrodynamic Force Measurement......Page 156 7.2.3 Trapping Potential Analysis......Page 158 7.3 Kinetic Potential Analysis......Page 159 7.4 Summary......Page 163 References......Page 164 8.2 Development of a Near-Infrared 35 fs Laser Microscope and its Application to Higher Order Multiphoton Excitation......Page 167 8.2.1 Confocal Microscope with a Chromium: Forsterite Ultrafast Laser as an Excitation Source......Page 168 8.2.2 Detection of Higher Order Multiphoton Fluorescence from Organic Crystals......Page 169 8.2.3 Multiphoton Fluorescence Imaging with the Near-Infrared 35 fs Laser Microscope......Page 171 8.3.1 Experimental System of FCS......Page 173 8.3.2 The Principle of the Method of Measurement of Local Temperature Using FCS......Page 174 8.3.3 Measurement of Local Temperature for Several Organic Solvents......Page 175 8.3.4 Summary......Page 180 8.4.1 Samples and Analysis of Experimental Data Obtained with FCS......Page 181 8.4.2 Non-Emissive Relaxation Dynamics in CdTe Quantum dots......Page 182 8.5 Summary......Page 184 References......Page 186 9.1 Introduction......Page 189 9.2 Nonlinear Optical Properties of CdTe QDs......Page 190 9.3 Optical Trapping of CdTe QDs Probed by Nonlinear Optical Properties......Page 192 9.4 Single Particle Spectroscopy of CdTe QDs......Page 196 9.5 Summary......Page 200 References......Page 201 Part Two Nanostructure Characteristics and Dynamics......Page 205 10.1 Introduction......Page 207 10.2.1 Significance of Photochemical Reactions......Page 208 10.2.3 Polymers with Spatially Graded Morphologies Designed from Photo-Induced Interpenetrating Polymer Networks (IPNs)......Page 209 10.2.4 Designing Polymers with an Arbitrary Distribution of Characteristic Length Scales by the Computer-Assisted Irradiation (CAI) Method......Page 211 10.2.5 Reversible Phase Separation Driven by Photodimerization of Anthracene: A Novel Method for Processing and Recycling Polymer Blends......Page 215 10.3 Concluding Remarks......Page 218 References......Page 219 11.1 Self-Organization and Self-Assembly......Page 221 11.2 Dissipative Structures......Page 223 11.3 Dynamics and Pattern Formation in Evaporating Polymer Solutions......Page 225 11.4 Applications of Dewetted Structures in Organic Photonics and Electronics......Page 230 References......Page 232 12.1 Introduction......Page 237 12.2 Position-Selective Arrangement of Nanosize Polymer Microspheres Onto a PS-b-P4VP Diblock Copolymer Film with Nanoscale Sea–island Microphase Structure......Page 239 12.3.2 Nanoscale Surface Morphological Change of PS-b-P4VP Block Copolymer Films Induced by Site-Selective Doping of a Photoactive Chromophore......Page 242 12.4 Site-Selective Modification of the Nanoscale Surface Morphology of Dye-Doped Copolymer Films Using Dopant-Induced Laser Ablation......Page 245 12.5 Photon Antibunching Behavior of Organic Dye Nanocrystals on a Transparent Polymer Film......Page 251 References......Page 255 13.1.1 Lipid Bilayer and its Fluidic Nature......Page 259 13.1.2 Controlling Molecular Diffusion in the Fluidic Lipid Bilayer......Page 261 13.1.3 Self-Spreading of a Lipid Bilayer or Monolayer......Page 263 13.1.4 Controlling the Self-Spreading Dynamics......Page 264 13.1.5 Molecular Manipulation on the Self-Spreading Lipid Bilayer......Page 267 13.2 Summary......Page 269 References......Page 270 14.1 Introduction......Page 273 14.2 Dynamic Self-Organization in Electrochemical Reaction Systems......Page 274 14.3 Oscillatory Electrodeposition......Page 275 14.3.1 Formation of a Layered Nanostructure of Cu–Sn Alloy......Page 276 14.3.2 Layered Nanostructures of Iron-Group Alloys......Page 280 14.3.3 Layered Nanostructure of Cu/Cu2O......Page 281 14.3.4 Nanostructured Metal Filaments......Page 284 14.4 Raman Microspectroscopy Study of Oscillatory Electrodeposition of Au at an Air/Liquid Interface......Page 286 14.5 Summary......Page 289 References......Page 290 15.1 Introduction......Page 293 15.2.1 Magnetic Orientation and Organization of SWNTs or their Composite Materials Using Polymer Wrapping......Page 294 15.2.2 Effects of Magnetic Processing on the Morphological, Electrochemical, and Photoelectrochemical Properties of Electrodes Modified with C60-Phenothiazine Nanoclusters......Page 298 15.2.3 Effects of Magnetic Processing on the Luminescence Properties of Monolayer Films with Mn2t-Doped ZnS Nanoparticles......Page 302 15.3.1 Magnetic Field Effects on the Dynamics of the Radical Pair in a C60 Clusters–Phenothiazine System......Page 304 15.3.2 Magnetic Field Effects on Photoelectrochemical Reactions of Electrodes Modified with the C60 Nanocluster-Phenothiazine System......Page 306 References......Page 308 16.1.1 Self-Assembled Monolayers......Page 313 16.1.2 Preparation of Gradient Surfaces......Page 314 16.1.3 Spontaneous Motion of a Droplet on Wetting Gradients......Page 315 16.1.4 Surface Switching......Page 316 16.2.1 Ratchet Motion of a Droplet on Asymmetric Electrodes......Page 318 16.2.2 Ratchet Motion of a Droplet Caused by Dynamic Motions of the Wetting Boundary......Page 319 16.3 Conclusion......Page 323 References......Page 325 17.1 Introduction......Page 327 17.2.1.1 Synthesis of CdSe Quantum Dots from Dimethyl Cadmium......Page 329 17.2.2 Synthesis of Water-Soluble Quantum Dots......Page 330 17.3 Bandgap Structure and Photoluminescence of CdSe Quantum Dots......Page 332 17.4 Photoluminescence Spectral Shifts......Page 333 17.4.1 Physical Effects on Spectral Shifts......Page 334 17.4.2 Chemical Effects on Spectral Shifts......Page 335 17.5 Enhancement of Photoluminescence in CdSe Quantum Dots......Page 337 17.6 On and Off Luminescence Blinking in Single Quantum Dots......Page 340 17.6.2 Modified Blinking......Page 342 References......Page 346 Volume II: Active Surfaces, Single Crystals and Single Biocells......Page 349 Contents to Volume 2......Page 355 Part Three Active Surfaces......Page 383 18.1 Introduction......Page 385 18.2.2 Computational Methods......Page 386 18.3.1 Dynamic Mechanism for Catalytic Dehydration of Formic Acid on a TiO2(110) Surface, Much Different from the Traditional Static Acid Catalysis......Page 387 18.3.2 Dynamic Catalytic Dehydrogenation of Formic Acid on a TiO2(110) Surface......Page 395 18.3.2.1 Mechanism of the Switchover of Reaction Paths......Page 399 18.4 Conclusion and Perspective......Page 400 References......Page 401 19.1 Introduction......Page 405 19.2.1.1 Principles......Page 406 19.2.1.2 Experimental Set-Up......Page 407 19.2.2.1 Principles and Brief History......Page 408 19.2.2.2 Experimental Set-Up......Page 409 19.3.1 Alkali Atom Desorption from a Metal Surface......Page 411 19.3.2 Solvation Dynamics at Metal Surfaces......Page 412 19.4.1 Vibrational Coherence and Coherent Phonons at Alkali-Covered Metal Surfaces......Page 413 19.4.2 Dephasing of the Vibrational Coherence: Excitation Fluence Dependence......Page 415 19.4.3 Excitation Mechanisms......Page 417 19.4.4 Mode Selective Excitation of Coherent Surface Phonons......Page 419 19.5 Concluding Remarks......Page 420 References......Page 421 20.1.1 Introduction......Page 425 20.1.2 Molecular Orbital Theory and Band Theory......Page 426 20.1.3 Charge Transfer vs. Charge Transport......Page 427 20.1.4 Electronic Excitation......Page 429 20.1.5 Reaction Dynamics......Page 431 20.2.1 Nonequilibrium Green's Function Formalism......Page 433 20.2.2 Efficient MO Approach......Page 435 20.2.3 Ab Initio Calculations: Single Molecular Conductance and Waveguide Effects......Page 438 20.2.4 Inelastic Transport and Inelastic Electron Tunneling Spectroscopy......Page 443 20.3.1 Theoretical Model of Hot Electron Transport and Reaction Probability......Page 449 20.3.2 Photodesorption Mechanism of Nitric Oxide on an Ag(111) Surface......Page 452 20.4 Summary and Outlook......Page 460 References......Page 462 21.1.1 NOx Reduction Technologies for Diesel and Lean-Burn Gasoline Engines......Page 469 21.1.2 Selective Catalytic Reduction of NOx by Hydrocarbons Over Ag/Al2O3......Page 470 21.2.1 Boosting of HC-SCR Activity of Ag/Al2O3 by Addition of H2......Page 471 21.2.2 Surface Dynamics of Ag Species Analyzed by in situ UV–Vis......Page 473 21.3.1 Reaction Scheme of HC-SCR Over Ag/Al2O3......Page 478 21.3.2 Effect of H2 Addition on Reaction Pathways of HC-SCR Over Ag/Al2O3......Page 482 21.4.1 Debates on Role of Ag Clusters......Page 484 21.4.2 Reductive Activation of O2 and Promoted HC-SCR on Ag Cluster......Page 488 References......Page 490 22.1 Introduction......Page 495 22.2 Formation and Structure of Highly Dispersed PdO Interacted with Brønsted Acid Sites......Page 496 22.3 Energy-Dispersive XAFS Studies on the Spontaneous Dispersion of PdO and Reversible Formation of Stable Pd Clusters in H-ZSM-5 and H-Mordenite......Page 498 22.4 In Situ QXAFS Studies on the Dynamic Coalescence and Dispersion Processes of Pd in USY Zeolite......Page 500 22.5 Time-Resolved EXAFS Measurement of the Stepwise Clustering Process of Pd Clusters at Room Temperature......Page 503 22.6 Summary......Page 506 References......Page 507 Part Four Single Crystals......Page 509 23.1 Introduction......Page 511 23.3 X-Ray Crystallographic Analysis......Page 512 23.4 Reactivity in the Crystal......Page 515 23.5 Photomechanical Effect......Page 516 23.6 Crystal Surface Changes......Page 517 23.7 Photoreversible Crystal Shape Changes......Page 518 References......Page 522 24.1.1 Crystal Engineering Renaissance......Page 527 24.2.1 Model of Photoisomerization......Page 528 24.2.2 Photoisomerization of Benzyl Muconate......Page 530 24.2.3 Change in Crystal Structures During Photoisomerization......Page 531 24.3.2 [2 + 2] Photodimerization of Benzyl Muconates......Page 533 24.4.1 Features of Topochemical Polymerization......Page 537 24.4.2 Monomer Stacking Structure and Polymerization Reactivity......Page 538 24.4.3 Shrinking and Expanding Crystals......Page 541 24.4.4 Accumulation and Release of Strain During Polymerization......Page 542 24.4.5 Homogeneous and Heterogeneous Polymerizations......Page 544 24.5 Conclusion......Page 548 References......Page 549 25.1 Introduction......Page 555 25.2 Photochromism of Rhodium Dithionite Complexes......Page 556 25.3.1 Dynamics of Molecular Structural Changes in Single Crystals......Page 558 25.3.2 Dynamics of Reaction Cavities in a Crystalline-State Reaction......Page 563 25.3.3 Dynamics of Surface Morphology Changes of Photochromic Single Crystals......Page 566 25.4 Summary......Page 567 References......Page 568 26.1 Introduction......Page 573 26.2.1 Guest-Responsive Molecular Assemblies......Page 574 26.2.2 Intercalation in Steroidal Bilayer Crystals......Page 576 26.2.3 Guest Fit Through Weak Non-Covalent Bonds......Page 578 26.3.1 Solid-State Fluorescence Emission......Page 580 26.3.2 Hydrogen Bond Clusters......Page 582 26.4.1 Hierarchical Structures with Supramolecular Chirality......Page 584 26.4.2.1 Three-Axial Chirality......Page 585 26.4.2.2 Tilt Chirality......Page 586 26.4.2.3 Helical and Bundle Chirality in a 21 Assembly......Page 587 26.4.3 Supramolecular Chirality of Hydrogen Bonding Networks......Page 588 26.4.4 Expression of Molecular Information......Page 590 References......Page 591 27.1 Introduction......Page 595 27.2.1 Solid-State Photocylization......Page 596 27.2.2 Crystal Structures and the Reaction Mechanism......Page 597 27.2.3 Morphology Changes in Bulk Crystals......Page 599 27.2.4 Morphology Changes in Microcrystals......Page 600 27.2.5 Correlation between the Morphology Changes and the Crystal Strucural Changes......Page 603 27.3.1 Solid-State Photocyclization and the Crystal Structures......Page 605 27.3.2 Morphology Changes......Page 607 References......Page 609 Part Five Single Biocells......Page 613 28.1 Introduction......Page 615 28.2 Femtosecond Laser Ablation and Generated Impulsive Force in Water: Laser Tsunami......Page 616 28.2.1 Manipulation of a Single Polymer Bead by Laser Tsunami......Page 619 28.2.2 Manipulation of Single Animal Cells by Laser Tsunami......Page 622 28.2.3 Modification and Regeneration Process in Single Animal Cells by Laser Tsunami......Page 624 28.2.4 Injection of Nanoparticles into Single Animal Cells by the Laser Tsunami......Page 626 28.3 Development of Rayleigh Light Scattering Spectroscopy/Imaging System and its Application to Single Animal Cells......Page 629 28.4 Summary......Page 633 References......Page 634 29.1.2 Super-Resolution Microscopy by Two-Color Double Resonance Spectroscopy......Page 639 29.1.3 Transient Fluorescence Detected IR Spectroscopy......Page 640 29.1.4 Application to Super-Resolution Infrared Microscopy......Page 641 29.2.2.1 Optical Layout for the Solution and Fluorescent Beads......Page 642 29.2.2.2 Optical Layout for Biological Samples......Page 643 29.3.1 Transient Fluorescence Image with IR Super-Resolution in Solution......Page 644 29.3.2 Picosecond Time-Resolved Measurement......Page 646 29.3.3 Application to Fluorescent Beads......Page 647 29.3.4.1 Super-Resolution IR Imaging of Arabidopsis thaliana Roots......Page 649 29.3.4.2 Vibrational Relaxation Dynamics in the Cells......Page 650 29.4 Summary......Page 652 References......Page 653 30.1.1 Thylakoid Membranes of Oxygenic Photosynthesis......Page 657 30.1.4 Applications of Fluorescence Microscopy to a Thylakoid Membrane......Page 658 30.1.5 Simultaneous Spectral Imaging and its Merits......Page 659 30.2.1 Realization of Fast Broadband Spectral Acquisition in Two-Photon Excitation Fluorescence Imaging......Page 660 30.2.2.2 Stability of the Anabaena Fluorescence Spectra Under Photoautotrophic Conditions......Page 662 30.2.2.3 Change of the Anabaena Fluorescence Spectra by Dark Conditions......Page 663 30.2.2.4 Intracellular Spectral Gradient in Anabaena Cells......Page 664 30.2.3.1 Chloroplasts from a Plant, Zea mays......Page 666 30.2.3.2 Chloroplast from the Green Alga, Chlorella......Page 668 30.3 Technical Verification and Perspective......Page 669 30.4 Summary......Page 670 References......Page 672 31.1 Introduction......Page 675 31.2.1 FLIM Measurement System......Page 676 31.2.3 Measurements of External Electric Field Effects......Page 678 31.3.1 FLIM of Hb. salinarum......Page 679 31.3.2 pH Dependence of the Fluorescence Lifetime in Solution and in Living Cells......Page 682 31.3.3 External Electric Field Effect on Fluorescence of BCECF......Page 684 31.3.4 Electric-Field-Induced Aggregate Formation in Hb. salinarum......Page 685 References......Page 687 32.1 Introduction......Page 691 32.2.1 Time-Gated Excitation–Emission Matrix Spectroscopy......Page 693 32.2.2 Time- and Spectrally-Resolved Fluorescence Imaging......Page 694 32.2.3 PARAFAC Model......Page 696 32.3.1 The 3D Fluorescence Properties of Dye Solutions......Page 698 32.3.2 The 3D Fluorescence Property of a Mixed Solution......Page 699 32.3.3 PARAFAC Decomposition Without any Prior Knowledge of Constituents......Page 701 32.4.1 Characterization of γ–Em Maps......Page 703 32.4.3 PARAFAC Decomposition......Page 705 32.4.4 Possible Assignments of Fluorescent Components......Page 707 32.5 Concluding Remarks......Page 708 References......Page 710 33.1.1 Investigation on Biological System Based on Molecular Identification and Visualization......Page 713 33.1.2.1 Spatial Resolution......Page 715 33.1.3 Time and Space Resolution Required to Observe Anomalous Diffusion of a Single Molecule in Biological Tissues......Page 716 33.1.4 General Importance of Anomalous Diffusion in a Signaling Reaction......Page 720 33.2.1 Use of FCS for Biological Systems......Page 723 33.2.2 Experimental Example of Anomalous Diffusion Observed in a Model System for Extracellular Matrices......Page 724 33.2.3 Quantitative Estimation of Reaction Volume in Signaling Reaction......Page 729 33.3.1 FCS Measurement Inside Single Cells......Page 730 33.4 Summary......Page 732 References......Page 733 34.1.1 Spectroscopic Properties of Gold Nanorods......Page 737 34.1.2 Biocompatible Gold Nanorods......Page 738 34.2.1 Gold Nanorods Targeting Tumor Cells......Page 742 34.2.2 Spectroscopy of Gold Nanorods In Vivo......Page 743 34.3 Photoreactions of Gold Nanorods for Biochemical Applications......Page 748 34.4 Conclusions and Future Outlook......Page 750 References......Page 751 35.1.1 Single Cell Analysis......Page 757 35.1.2 Dynamic Motion of Murine Embryonic Stem Cell......Page 758 35.2.1 Optical Tweezers......Page 759 35.2.2 Set-up for Optical Trapping of a Living Cell......Page 760 35.2.3 Murine Embryonic Stem Cell Trapped with Optical Tweezers......Page 761 35.3.1 Dynamic Motion of a Murine Embryonic Stem Cell......Page 762 35.3.2 Experimental Procedure......Page 763 35.4.1 Cell Separation......Page 767 35.5 Summary......Page 768 References......Page 769 Index......Page 771 |
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