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題目Au–Pd alloy nanoparticle catalyzed selective oxidation of benzyl alcohol and tandem synthesis of imines at ambient conditions 作者Wenjing Cui, Qi Xiao, Sarina Sarina 其他Catalysis Today, Volume 235, 15 October 2014, Pages 152-159 |
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https://apps.webofknowledge.com/ ... age=1&doc=1 Au-Pd alloy nanoparticle catalyzed selective oxidation of benzyl alcohol and tandem synthesis of imines at ambient conditions 作者:Cui, WJ (Cui, Wenjiang)[ 1,2 ] ; Xiao, Q (Xiao, Qi)[ 3 ] ; Sarina, S (Sarina, Sarina)[ 3 ] ; Ao, WL (Ao, Wulan)[ 1 ] ; Xie, MX (Xie, Mengxia)[ 4 ] ; Zhu, HY (Zhu, Huaiyong)[ 3 ] ; Bao, Z (Bao, Zhaorigetu)[ 1 ] CATALYSIS TODAY 卷: 235 頁: 152-159 DOI: 10.1016/j.cattod.2014.04.015 出版年: OCT 15 2014 查看期刊信息 CATALYSIS TODAY 出版商 ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS ISSN: 0920-5861 eISSN: 1873-4308 研究領(lǐng)域 Chemistry Engineering 摘要 Alloy nanoparticles (NPs) of gold and palladium on ZrO2 support (Au-Pd@ZrO2) were found to be highly active in oxidation of benzyl alcohols and can be used for the tandem synthesis of imines from benzyl alcohols and amines via a one-pot, two-step process at mild reaction conditions. The first step of the process is oxidation of benzyl alcohol to benzaldehyde, excellent yields were achieved after 7 h reaction at 40 degrees C without addition of any base. In the second step, aniline was introduced into the reaction system to produced N-benzylideneaniline. The benzaldehyde obtained in the first step was completely consumed within 1 h. A range of benzyl alcohols and amines were investigated for the general applicability of the Au-Pd alloy catalysts. It is found that the performance of the catalysts depends on the Au-Pd metal contents and composition. The optimal catalyst is 3.0 wt% Au-Pd@ZrO2 with a Au  d molar ratio 1:1. The alloy NP catalyst exhibited superior catalytic properties to pure AuNP or PdNP because the surface of alloy NPs has higher charge heterogeneity than that of pure metal NPs according to simulation of density function theory (DFT). (C) 2014 Elsevier B.V. All rights reserved.關(guān)鍵詞 作者關(guān)鍵詞:Tandem synthesis; Gold and palladium alloy nanoparticles; Benzyl alcohol; Amine; Imine KeyWords Plus:SUPPORTED GOLD NANOPARTICLES; SOLVENT-FREE OXIDATION; BIMETALLIC CATALYSTS; AEROBIC OXIDATION; MOLECULAR-OXYGEN; PALLADIUM; AMINES; MECHANISM; SIEVES 作者信息 通訊作者地址: Zhu, HY (通訊作者) Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia. 增強組織信息的名稱 Queensland University of Technology 地址: [ 1 ] Inner Mongolia Normal Univ, Inner Mongolia Key Lab Green Catalysis, Hohhot 010022, Inner Mongolia, Peoples R China 增強組織信息的名稱 Inner Mongolia Normal University [ 2 ] Inner Mongolia Vocat Coll Chem Engn, Dept Chem Engn, Hohhot 010070, Inner Mongolia, Peoples R China [ 3 ] Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia 增強組織信息的名稱 Queensland University of Technology [ 4 ] Beijing Normal Univ, Analyt Testing Ctr, Beijing 100875, Peoples R China 增強組織信息的名稱 Beijing Normal University 電子郵件地址:hy.zhu@qut.edu.au; zrgt@imnu.edu.cn 基金資助致謝 基金資助機構(gòu) 授權(quán)號 National Natural Science Foundation of China 20966008 Opening Project of Natural Science Foundation of Inner Mongolia 2010KF02 Australia Research Council ARC DP110104990 查看基金資助信息關(guān)閉基金資助信息 Financial supports from the National Natural Science Foundation of China (No. 20966008), Opening Project of Natural Science Foundation of Inner Mongolia (No. 2010KF02) and Australia Research Council (ARC DP110104990) are gratefully acknowledged. 出版商 ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS 類別 / 分類 研究方向:Chemistry; Engineering Web of Science 類別:Chemistry, Applied; Chemistry, Physical; Engineering, Chemical 文獻信息 文獻類型:Article 語種:English 入藏號: WOS:000340946200018 ISSN: 0920-5861 eISSN: 1873-4308 其他信息 IDS 號: AN9RP Web of Science 核心合集中的 "引用的參考文獻": 42 Web of Science 核心合集中的 "被引頻次": 2 JCR® 類別 JCR 分區(qū) CHEMISTRY, APPLIED Q1 CHEMISTRY, PHYSICAL Q2 ENGINEERING, CHEMICAL Q1 數(shù)據(jù)來自第 2013 版 Journal Citation Reports® |
2樓2015-04-21 20:25:21
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zczcwj: 金幣+10, ★★★★★最佳答案 2015-04-21 20:33:21
心靜_依然: LS-EPI+1, 感謝應(yīng)助 2015-04-21 20:45:48
zczcwj: 金幣+10, ★★★★★最佳答案 2015-04-21 20:33:21
心靜_依然: LS-EPI+1, 感謝應(yīng)助 2015-04-21 20:45:48
| 入藏號: WOS:000340946200018 |
3樓2015-04-21 20:25:33
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